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Application of 940 nm high-power DFB lasers for line-broadening measurements at normal pressure using a robust and compact setup

B. Sumpf, A. Klehr, G. Erbert, G. Tränkle

Published in:

Appl. Phys. B, vol. 106, no. 2, pp. 357-364 (2012).

Abstract:

High-power distributed-feedback (DFB) lasers for the wavelength range near 940 nm (i.e. about 10,600 cm-1) were used for line-broadening measurements of individual rotational-vibrational absorption lines of water vapour at atmospheric pressure using a minimalist set-up. The laser has a maximum output power larger than 500 mW. Over the whole power range from threshold to maximum power, it operates in single mode operation with a tuning range of 4.7 nm, i.e. 50 cm-1, at 20°C. With an emission line-width ≤2 MHz (0.66×10-4 cm-1), the device is well suited for high-resolution spectroscopy.
Instead using a sophisticated optical set-up with a multi-reflection cell to obtain the necessary path length for measuring rather weak absorption lines, in this work a 4" integrating sphere was used as a multi-reflection cell providing an effective absorption length of 6.7 m. The laser was placed without any optical elements in front of the entrance hole.
The power-current-characteristics, the spectral features of the diode laser, and examples for the spectral tuning will be given. In the spectral range from 10,584.3 cm-1 to 10,670.2 cm-1, line broadening coefficients in the range 0.059 cm-1/atm ≤ γH2O-air ≤ 0.112 cm-1/atm were measured for 18 H2O absorption lines from the 2ν13-band and 7 H2O lines from the 3ν1-band. The good agreement of the measured air-broadening coefficients with data from the literature for absorption lines with a J"≤4 and Ka"≤3 proves the applicability of this low-cost set-up. Some deviations between the literature and this work were observed for lines from the 2ν13-band with larger J">4 and Ka"=3.

Ferdinand-Braun-Institut, Leibniz-Institut für Höchstfrequenztechnik, Gustav-Kirchhoff-Straße 4, D-12489 Berlin, Germany

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